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2018 Vol.28, Issue 9
Enhanced Piezoelectric Properties of (1−x)[0.675BiFeO3−0.325BaTiO3]−xLiTaO3 Ternary System by Air-Quenching
Fazli Akram1
,
Rizwan Ahmed Malik12
,
Soonil Lee1
,
Riffat Asim Pasha2
,
Myong Ho Kim1†
1School of Materials Science and Engineering, Changwon National University, Gyeongnam 51140, Republic of Korea
2Department of Metallurgy and Materials Engineering, UET Taxila, Taxila, Pakistan
†Corresponding author E-Mail : mhkim@changwon.ac.kr (M.-H. Kim, Changwon Nat’l Univ.)
September 2018. pp. 489-494
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Abstract

Lead free (1-x)(0.675BiFeO3-0.325BaTiO3)- xLiTaO3 (BFBTLT, x = 0, 0.01, 0.02, and 0.03, with 0.6 mol% MnO2 and 0.4 mol% CuO) were prepared by a solid state reaction method, followed by air quenching and their crystalline phase, morphology, dielectric, ferroelectric and piezoelectric properties were explored. An X-ray diffraction study indicates that lithium (Li) and tantalum (Ta) were fully incorporated in the BFBT materials with the absence of any secondary phases. Dense ceramic samples (> 92 %) with a wide range of grain sizes from 3.70 μm to 1.82 μm were obtained in the selected compositions (0 ≤ x ≤ 0.03) of BFBTLT system. The maximum temperatures (Tmax) were mostly higher than 420 °C in the studied composition range. The maximum values of maximum polarization (Pmax ≈ 31.01 μC/cm2), remnant polarization (Prem ≈ 22.82 μC/cm2) and static piezoelectric constant (d33 ≈ 145 pC/N) were obtained at BFBT-0.01LT composition with 0.6 mol% MnO2 and 0.4 mol% CuO. This study demonstrates that the high Tmax and d33 for BFBTLT ceramics are favorable for industrial applications.

Keywords
lead-free
bismuth ferrite
dielectric
ferroelectric
piezoelectric
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Information
  • Publisher :Materials Research Society of Korea
  • Publisher(Ko) :한국재료학회
  • Journal Title :Korean Journal of Materials Research
  • Journal Title(Ko) :한국재료학회지
  • Volume : 28
  • No :9
  • Pages :489-494
  • Received Date : 2018-08-17
  • Revised Date : 2018-08-20
  • Accepted Date : 2018-08-31
  • DOI :https://doi.org/10.3740/MRSK.2018.28.9.489
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